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Trigonal Planar [HgSe3]4– Unit: A New Kind of Basic Functional Group in IR Nonlinear Optical Materials with Large Susceptibility and Physicochemical Stability
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Update time: 2016-05-22
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A new mercury selenide BaHgSe2 was synthesized. This air-stable compound displays a large nonlinear optical (NLO) response and melts congruently. The structure contains chains of corner-sharing [HgSe3]4– anions in the form of trigonal planar units, which may serve as a new kind of basic functional group in IR NLO materials to confer large NLO susceptibilities and physicochemical stability. Such trigonal planar units may inspire a path to finding new classes of IR NLO materials of practical utility that are totally different from traditional chalcopyrite materials.

J. Am. Chem. Soc., 2016, 138 (19), pp 6135–6138
 

 

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